Innovative Spektroskopien in der f-Element Chemie
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Abteilungsleiter: Prof. Dr. Tonya Vitova
+49 721 608 24024 |
Die Abteilung unter der Leitung von Prof. Dr. Tonya Vitova untersucht in systematischer Weise die elektronische und koordinative Struktur sowohl von Actinid (An)-Verbindungen, als auch von chemisch homologen Lanthaniden (Ln). Hierbei kommen die auf Synchrotronstrahlung basierenden innovativen Methoden der hochauflösenden Röntgenfluoreszenzemission (HRXES) und der inelastischen Röntgenstreuung (RIXS) zum Einsatz. Experimentelle Ergebnisse werden durch Vergleich mit theoretischen Rechnungen und Simulationen auf der Basis quantenchemischer Verfahren interpretiert. Das Ziel der Untersuchungen ist eine Verbesserung des Verständnisses der Reaktivität von An/Ln-Species auf molekularer Ebene in den verschiedenen technischen und geologischen Barrieren eines Endlagers, um hierdurch die Zuverlässigkeit von Modellrechnungen zur Langzeitsicherheit zu erhöhen. Die Aufklärung der elektronischen und der Koordinations-Struktur von An- und Ln-Systemen gewährt eine grundlegende Einsicht in den Zusammenhang von elektronischer Struktur und chemischer Reaktivität von Actinid-Elementen.
Members
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Tonya Vitova Teaching activities:
E-Mail: tonya.vitova∂kit.edu |
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Bianca Schacherl Development of X-ray Spectroscopies and Radiochemical Applications E-Mail: bianca.schacherl∂kit.edu |
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Harry Ramanantoanina Theoretical Spectroscopy E-Mail: harry.ramanantoanina∂kit.edu |
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Jacob Branson Since Jan. 2025 E-Mail: jacob.branson∂kit.edu |
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Christian Vollmer Since 2021 E-Mail: christian.vollmer∂kit.edu |
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Cedric Reitz Since May 2023 E-Mail: cedric.reitz∂kit.edu |
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Hanna Kaufmann-Heimeshoff Since Nov. 2023 |
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Emily Reynolds Since Jul. 2024 E-Mail: emily.reynolds∂kit.edu |
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Kiara Maurer Since Nov. 2024 E-Mail: kiara.maurer∂student.kit.edu |
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Sven Schenk Since Jan. 2025 E-Mail: sven.schenk∂kit.edu |
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Vivek Sharma Since Oct. 2024 |
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Samantha Bratzel Since Jan. 2025 |
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Ruwini Ekanayake, Karlsruhe Institute of Technology (KIT), Germany 01.03.2023 - 01.09.2024: Post Doc project “Advanced X-ray spectroscopy development”
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Xiaobin Zhang, Karlsruhe Institute of Technology (KIT), Germany 01.01.2023 - 01.06.2024: Post Doc project “Theoretical chemistry and bond analysis”
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Chaerin Kim, South Korea 01.10.2023 - 01.03.2024: Exchange student project “Lanthanide spectroscopy”
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Natalia Müller, Karlsruhe Institute of Technology (KIT), Germany 15.05.2021 - 01.06.2023: Post Doc project “High resolution ligand spectroscopy of actinide systems”
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Thomas Neill, University of Manchester, UK 2019 - 2021 : Post Doc project “The aquatic chemistry and electronic structure properties of actinides using high-resolution X-ray methods.”
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Christian Vollmer, Karlsruhe Institute of Technology (KIT), Germany
1.02.2021 – 30.08.2021 : Master thesis “Advanced uranium M4,5-edge X-ray spectroscopic investigations of uranium carbonate species in solid and liquid state in multiple oxidation states”” |
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Jurij Galanzew, Karlsruhe Institute of Technology (KIT), Germany
09.2017 - 03.2018: Master thesis “Electronic structure studies of Th systems by high energy resolution X-ray spectroscopy and computational methods” PhD Project: "High energy resolution X-ray spectroscopy and computational studies of Uranium interaction with magnetite and siderite" |
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Aaron Beck, Karlsruhe Institute of Technology (KIT), Germany
12.2016 - 06.2017: Master thesis “Immobilization of cesium- and rhenium-rich simulated high level solid waste residues in different host matrices” PhD Project: "High energy resolution X-ray spectroscopy investigations of nuclear waste" |
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Sebastian Bahl, Karlsruhe Institute of Technology (KIT), Germany 2013 - 2017: PhD project “Characterisation of nuclear waste glass forms by advanced spectroscopy and microscopy techniques” 02.2013 - 07.2013: Diploma thesis „Charakterisierung von verglasten, hochradioaktiven, Mo/P/Zr/Cs-reichen Simulatabfällen mittels verschiedener spektroskopischer Techniken“, Grade: 1.0 (highest in Germany) |
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Alisa Prokopchuk, Karlsruhe Institute of Technology (KIT), Germany
10.2016 - 04.2017: Master thesis „Preparation of Rb2UO2X4 compounds (X= F,Cl,Br) and characterizytion of bonding differences by spectroscopy and quantum chemical methods“ |
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Ivan Pidchenko, Institut für Nukleare Entsorgung, Karlsruhe Institute of Technology (KIT), Germany
10.2016 - 04.2017: PhD project 2017 - Postdoc „Characterisation of actinide species in systems relevant for safety assessment of a nuclear waste repository by high-resolution X-ray emission/absorption spectroscopy“ |
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Tim Prüßmann, Institut für Nukleare Entsorgung, Karlsruhe Institute of Technology (KIT), Germany
07.2011 - 04.2015: PhD project „Characterization of bonding differences by advanced synchrotron based X-ray spectroscopy“ |
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Veronika Koldeisz, Budapest University of Technology and Economics (BME), Hungary
09.2013 – 07.2014: Master's thesis “Characterization of uranium in multi-component borosilicate glass by high-energy resolution X-ray spectroscopy techniques”, Grade: 5.0 (highest in Hungary) |
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Paul Estevenon, École Nationale Supérieure de Chimie de Montpellier (ENSCM), France
06.2014 - 09.2014: Internship "Characterization of simulated Tc- and Cs-rich solid waste residue" |
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Andrea Kutzer, Karlsruhe Institute of Technology (KIT), Germany
2011 - 2014: PhD project “Untersuchungen zum Inkorporationsverhalten von simulierten HLW-Borosilikatgläsern zur Immobilisierung Mo(VI)-reicher Abfälle”
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Alexander Ernst, Karlsruhe Institute of Technology (KIT)
04.2012 - 09.2012: practical part of “berufliche Ausbildung” "Design and technical drawings of positioning part of a detector positioning assembly"
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Valentine Traunfelder, Karlsruhe Institute of Technology (KIT)
04.2013 – 01.2014: practical part of “berufliche Ausbildung” “Design and technical drawings of liquid cells for M edge high resolution X-ray absorption spectroscopy studies of actinide materials”
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Heloise Morin, École des Mines de Nantes (Mines Nantes), France
05.2011 - 08.2011 “Measurements, data reduction and comparison of N K-edge XANES spectra of n-Pr-BTP ligand and [Ln(n-Pr-BTP)3](NO3)3 complexes”
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Bastien Gademann, National Graduate School of Chemistry of Montpellier (ENSCM), France
06.2012 - 09.2012 “Alignment procedure of a multi-analyzer crystal X-ray emission spectrometer using SPEC macros”
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Stelyana Lechchanska, Technical University of Sofia (TU Sofia), Bulgaria
07.2013 - 09.2013 “Design and technical drawings of a slit system, an integral part of the multi-analyzer crystals X-ray emission spectrometer”
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Aurora Walesh, Trinity Collage Dublin (TCD), School of Chemistry, Ireland
4.03.2013 - 15.03.2013: Short term scientific mission “Structural characterization of UO2 alteration products by X-ray techniques” Funded by COST: European cooperation in science and technology |
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Yulia Podkovyrina, Southern Federal University (SFedU) Rostov-on-Don, Russia
02.2014 –03.2014: Scholarship “Quantum chemical calculations of HR-XANES M edge spectra of uranium oxides” Funded by German Russian Interdisciplinary Science Center (G-RISC) 10.2014 –03.2015: Scholarship “Optimization of structures describing U sorption and incorporation into magnetite” Funded by German Academic Exchange Service (DAAD) |
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Prof. Robert Baker, Trinity College Dublin (TCD), School of Chemistry, Ireland
01.2015- 03.2015: TALISMAN project “Neptunium Incorporation into Minerals: A Synthetic and X-ray Spectroscopic Study” |
Mar. 2025 : "Travel Award for the iSRS 2025 conference in Australia" |
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Congratulations! Kiara Maurer was awarded with the iSRS 2025 Travel Award for the iSRS 2025 conference in Australia this year by the SRS Education Committee.
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Feb. 2025 : "Our new Nature Communications paper is featured in KIT" |
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https://www.kit.edu/kit/pi_2025_007_actinide-neue-messmethode-klaert-bindungsverhaeltnisse.php |
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Jan. 2025 : "New Department at KIT/INE" |
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We are proud to anounce our new department "Advanced spectroscopy in f-element chemistry |
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Oct. 2024 : "ATAS – AnXAS 2024 best poster award" |
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Congratulations! Emily Reynolds got the best poster award award for her presentation "Development and Application of a Microfluidic Set-Up for In-Situ Studies of Formation Kinetics of La- and U-Complexes Using High Resolution Spectroscopic Methods" |
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Feb. 2024 : New group photo |
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Jul. 2024 : Cover of JACS |
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Jul. 2023 : Cover of Environmental Science & Technology |
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2023 : "Winners of the 16th KIT Doctoral Award of the year 2022/2023" |
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Congratulations! Bianca Schacherl got the KIT PHD award for her thesis "Advancing actinide high-enery resolution x-ray absorption/emission spectroscopy tools" |
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2023 : Cover of Inorganic Chemistry June 2023 |
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2023 : Bianca Schacherl receives ISTR-2023 Young Investigator Award |
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The ISTR-2023 Young Investigator Award handed over to B. Schacherl by former INE researcher M. A. Denecke.
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Bianca Schacherl has received the "Young Investigator Award” at the International Symposium on Trends in Radiopharmaceuticals (ISTR-2023) - organized by IAEA and held in Vienna, Austria, 17–21 April 2023. The poster contribution "Toward Understanding 225Ac3+ Radionuclide Bonding Properties within Radiopharmaceuticals: The Study of La3+ Homologues" was honored by the Technical Programme Committee of the Symposium headed by Ms. Najat Mokhtar, IAEA Deputy Director General and Head of the Department of Nuclear Sciences and Applications. |
Oct. 2022 : Our projects A1 and A3 are funded as part of the 4f for future CRC |
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A1 - Activation and Stabilization of Small Molecules by Rare-Earth Compounds
A3 - Lanthanide-Based Multimetallic Clusters: Impact of f-Elements on Formation, Structures, Electronic Properties and Reactivity |
2022: EDGE article - The mechanism of Fe induced bond stability of uranyl(v), Tonya Vitova, Laurent Maron, Marinella Mazzanti et al. |
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https://pubs.rsc.org/en/journals/journalissues/sc
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2020-2022: We upgraded our experimental set-up and can measure now actinide M4,5 edge HR-XANES spectra for geochemical samples containing 1 ppm of the actinide element at cryogenic temperatures. |
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2020 : Success with the proposal ERC Consolidator Grant 2020! |
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The ACTINIDE BOND properties in gas, liquid and solid state
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2017 and 2019: We made available new spectroscopy approaches and gained new insights into the covalency of the chemical bonding of the most studied molecules in actinide science - the actinyls |
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2017 and 2019: First An M4,5 HR-XANES and RIXS electronic and geometric structure studies probing the 5f unoccupied states of systems in liquid and solid states containing transuranium elements like Pu and Np |
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doi:10.1021/acs.inorgchem.7b02118
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2017: Applying the U M4 HR-XANES method, we demonstrated that U(V) can be stable in magnetite even in air |
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Invitation to the themed collection: New molecules and materials from the f-block of ChemComm |
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Invitation to the Inorganic Chemistry forum: Innovative f-Element Chelating Strategies |
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doi:10.1021/acs.inorgchem.9b02463
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Projects and Funding
THE ACTINIDE BOND : "Actinide bond properties in gas, liquid and solid state" |
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SFB : "4f for future" |
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InnoAlpha : "Innovative Concepts for Alpha-emitting Radionuclide Generators and Spectroscopy for Nuclear Medical Research and Applications" |
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NEXT : "NEXT generation probe of chemical bonding properties of actinides and lanthanides" |
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QUASY : "Quantum Sensor Platform for Synchrotron X-ray Spectroscopy" |
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ROXS : "Radionuclide Materials Observed with Soft X-ray Spectroscopy" |
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Publications
Schacherl, B.; Tagliavini, M.; Kaufmann-Heimeshoff, H.; Göttlicher, J.; Mazzanti, M.; Popa, K.; Walter, O.; Pruessmann, T.; Vollmer, C.; Beck, A.; Ekanayake, R. S. K.; Branson, J. A.; Neill, T.; Fellhauer, D.; Reitz, C.; Schild, D.; Brager, D.; Cahill, C.; Windorff, C.; Sittel, T.; Ramanantoanina, H.; Haverkort, M. W.; Vitova, T.
2025. Nature Communications, 16 (1), Article no: 1221. doi:10.1038/s41467-024-54574-7
Bagus, P. S.; Nelin, C. J.; Schacherl, B.; Vitova, T.; Polly, R.
2024. The Journal of Physical Chemistry A, 128 (38), 8024–8034. doi:10.1021/acs.jpca.4c03555
Vitova, T.; Ramanantoanina, H.; Schacherl, B.; Münzfeld, L.; Hauser, A.; Ekanayake, R. S. K.; Reitz, C. Y.; Prüßmann, T.; Neill, T. S.; Göttlicher, J.; Steininger, R.; Saveleva, V. A.; Haverkort, M. W.; Roesky, P. W.
2024. Journal of the American Chemical Society, 146 (30), 20577–20583. doi:10.1021/jacs.3c13934
Bagus, P. S.; Nelin, C. J.; Schacherl, B.; Vitova, T.
2024. Inorganic Chemistry, 63 (29), 13202 – 13213. doi:10.1021/acs.inorgchem.4c00270
Yu, Y.; Hao, Y.; Xiao, B.; Langer, E.; Novikov, S. A.; Ramanantoanina, H.; Pidchenko, I.; Schild, D.; Albrecht-Schoenzart, T. E.; Eichel, R.-A.; Vitova, T.; Alekseev, E. V.
2024. Chemistry – A European Journal, 30 (40), Art.-Nr.: e202401033. doi:10.1002/chem.202401033
Brown, A. R.; Molinas, M.; Roebbert, Y.; Faizova, R.; Vitova, T.; Sato, A.; Hada, M.; Abe, M.; Mazzanti, M.; Weyer, S.; Bernier-Latmani, R.
2024. Geochemical Perspectives Letters, 29, 45–50. doi:10.7185/geochemlet.2411
Ehrman, J. N.; Shumilov, K.; Jenkins, A. J.; Kasper, J. M.; Vitova, T.; Batista, E. R.; Yang, P.; Li, X.
2024. JACS Au, 4 (3), 866–1249. doi:10.1021/jacsau.3c00838
Faden, L.-P.; Reiß, A.; Popescu, R.; Donsbach, C.; Göttlicher, J.; Vitova, T.; Gerthsen, D.; Feldmann, C.
2024. Inorganic Chemistry, 63 (2), 1020–1034. doi:10.1021/acs.inorgchem.3c03074
Bagus, P. S.; Nelin, C. J.; Rosso, K. M.; Schacherl, B.; Vitova, T.
2024. Inorganic Chemistry, 63 (4), 1793–1802. doi:10.1021/acs.inorgchem.3c03158
Butorin, S. M.; Bauters, S.; Amidani, L.; Beck, A.; Rossberg, A.; Weiss, S.; Vitova, T.; Kvashnina, K. O.; Tougait, O.
2023. Scientific Reports, 13 (1), Art-Nr.: 20434. doi:10.1038/s41598-023-47579-7
Schacherl, B.; Joseph, C.; Beck, A.; Lavrova, P.; Schnurr, A.; Dardenne, K.; Geyer, F.; Cherkezova-Zheleva, Z.; Göttlicher, J.; Geckeis, H.; Vitova, T.
2023. Environmental Science and Technology, 57 (30), 11185–11194. doi:10.1021/acs.est.2c09356
Vigier, J.-F.; Wiss, T.; Palina, N.; Vitova, T.; Colle, J.-Y.; Bouëxière, D.; Freis, D.; Konings, R. J. M.; Popa, K.
2023. Inorganic Chemistry, 62 (24), 9350–9359. doi:10.1021/acs.inorgchem.3c00251
Kiefer, C.; Neill, T.; Cevirim-Papaioannou, N.; Schild, D.; Gaona, X.; Vitova, T.; Dardenne, K.; Rothe, J.; Altmaier, M.; Geckeis, H.
2022. Frontiers in Chemistry, 10, Art.-Nr.: 1042709. doi:10.3389/fchem.2022.1042709
Kalt, J.; Sternik, M.; Sergeev, I.; Mikolasek, M.; Bessas, D.; Göttlicher, J.; Krause, B.; Vitova, T.; Steininger, R.; Sikora, O.; Jochym, P. T.; Leupold, O.; Wille, H.-C.; Chumakov, A. I.; Piekarz, P.; Parlinski, K.; Baumbach, T.; Stankov, S.
2022. Physical Review B, 106 (20), Article no: 205411. doi:10.1103/PhysRevB.106.205411
Vigier, J.-F.; Freis, D.; Walter, O.; Dieste Blanco, O.; Bouëxière, D.; Zuleger, E.; Palina, N.; Vitova, T.; Konings, R. J. M.; Popa, K.
2022. CrystEngComm, 24 (36), 6338–6348. doi:10.1039/d2ce00527a
Vitova, T.; Faizova, R.; Amaro-Estrada, J. I.; Maron, L.; Pruessmann, T.; Neill, T.; Beck, A.; Schacherl, B.; Tirani, F. F.; Mazzanti, M.
2022. Chemical Science, 13 (37), 11038–11047. doi:10.1039/D2SC03416F
Butorin, S. M.; Bauters, S.; Amidani, L.; Beck, A.; Weiss, S.; Vitova, T.; Tougait, O.
2022. Journal of Synchrotron Radiation, 29 (2), 295–302. doi:10.1107/S160057752101314X
Köhler, L.; Patzschke, M.; Bauters, S.; Vitova, T.; Butorin, S. M.; Kvashnina, K. O.; Schmidt, M.; Stumpf, T.; März, J.
2022. Chemistry - A European Journal, 28 (21), Art.-Nr. e202200119. doi:10.1002/chem.202200119
Sun, J.; Zhou, J.; Li, L.; Hu, Z.; Chan, T.-S.; Vitova, T.; Song, S.; Liu, R.; Jing, C.; Yu, H.; Zhang, M.; Rothe, J.; Wang, J.-Q.; Zhang, L.
2022. Chemical Communications, 58 (21), 3469–3472. doi:10.1039/d2cc00576j
Schacherl, B.; Joseph, C.; Lavrova, P.; Beck, A.; Reitz, C. Y.; Prüssmann, T.; Fellhauer, D.; Lee, J.-Y.; Dardenne, K.; Rothe, J.; Geckeis, H.; Vitova, T.
2022. Analytica chimica acta, 1202, Art.Nr.: 339636. doi:10.1016/j.aca.2022.339636
Pan, Z.; Roebbert, Y.; Beck, A.; Bartova, B.; Vitova, T.; Weyer, S.; Bernier-Latmani, R.
2022. Environmental Science and Technology, 56 (3), 1753–1762. doi:10.1021/acs.est.1c06865
Vitova, T.; Roesky, P. W.; Dehnen, S.
2022. Communications chemistry, 5, Art.-Nr. 12. doi:10.1038/s42004-022-00630-6
Prüßmann, T.; Nagel, P.; Simonelli, L.; Batchelor, D.; Gordon, R.; Schimmelpfennig, B.; Trumm, M.; Vitova, T.
2022. Journal of synchrotron radiation, 29 (1), 53–66. doi:10.1107/S1600577521012091
Schacherl, B.; Prüssmann, T.; Dardenne, K.; Hardock, K.; Krepper, V.; Rothe, J.; Vitova, T.; Geckeis, H.
2022. Journal of synchrotron radiation, 29 (1), 80–88. doi:10.1107/S1600577521012650
Kumar, S.; Rothe, J.; Finck, N.; Vitova, T.; Dardenne, K.; Beck, A.; Schild, D.; Geckeis, H.
2022. Colloids and surfaces / A, 635, Article no: 128105. doi:10.1016/j.colsurfa.2021.128105
Stagg, O.; Morris, K.; Lam, A.; Navrotsky, A.; Velázquez, J. M.; Schacherl, B.; Vitova, T.; Rothe, J.; Galanzew, J.; Neumann, A.; Lythgoe, P.; Abrahamsen-Mills, L.; Shaw, S.
2021. Environmental Science and Technology, 55 (24), 16445–16454. doi:10.1021/acs.est.1c06197
Polly, R.; Schacherl, B.; Rothe, J.; Vitova, T.
2021. Inorganic chemistry, 60 (24), 18764–18776. doi:10.1021/acs.inorgchem.1c02364
Bagus, P. S.; Schacherl, B.; Vitova, T.
2021. Inorganic chemistry, 60 (21), 16090–16102. doi:10.1021/acs.inorgchem.1c01331
Suksi, J.; Tullborg, E.-L.; Pidchenko, I.; Krall, L.; Sandström, B.; Kaksonen, K.; Vitova, T.; Kvashnina, K. O.; Göttlicher, J.
2021. Chemical Geology, 584, Art.-Nr.: 120551. doi:10.1016/j.chemgeo.2021.120551
Prieur, D.; Vigier, J.-F.; Popa, K.; Walter, O.; Dieste, O.; Varga, Z.; Beck, A.; Vitova, T.; Scheinost, A. C.; Martin, P. M.
2021. Inorganic Chemistry, 60 (19), 14550–14556. doi:10.1021/acs.inorgchem.1c01071
Chevreux, P.; Tissandier, L.; Laplace, A.; Vitova, T.; Bahl, S.; Guyadec, F. L.; Deloule, E.
2021. Journal of nuclear materials, 544, Art.-Nr.: 152666. doi:10.1016/j.jnucmat.2020.152666
Kaiser, M.; Göttlicher, J.; Vitova, T.; Hinz, A.
2021. Chemistry - a European journal, 27 (30), 7998–8002. doi:10.1002/chem.202100888
Molinas, M.; Faizova, R.; Brown, A.; Galanzew, J.; Schacherl, B.; Bartova, B.; Meibom, K. L.; Vitova, T.; Mazzanti, M.; Bernier-Latmani, R.
2021. Environmental Science and Technology, 55 (8), 4753–4761. doi:10.1021/acs.est.0c06633
Townsend, L. T.; Morris, K.; Harrison, R.; Schacherl, B.; Vitova, T.; Kovarik, L.; Pearce, C. I.; Mosselmans, J. F. W.; Shaw, S.
2021. Chemosphere, 276, Art.-Nr.: 130117. doi:10.1016/j.chemosphere.2021.130117
Gerber, E.; Romanchuk, A. Y.; Weiss, S.; Bauters, S.; Schacherl, B.; Vitova, T.; Hübner, R.; Shams Aldin Azzam, S.; Detollenaere, D.; Banerjee, D.; Butorin, S. M.; Kalmykov, S. N.; Kvashnina, K. O.
2021. Inorganic Chemistry Frontiers, 8 (4), 1102–1110. doi:10.1039/d0qi01140a
Kegler, P.; Pointurier, F.; Rothe, J.; Dardenne, K.; Vitova, T.; Beck, A.; Hammerich, S.; Potts, S.; Faure, A.-L.; Klinkenberg, M.; Kreft, F.; Niemeyer, I.; Bosbach, D.; Neumeier, S.
2021. MRS advances, 6, 126–134. doi:10.1557/s43580-021-00024-1
Kalt, J.; Sternik, M.; Krause, B.; Sergueev, I.; Mikolasek, M.; Merkel, D.; Bessas, D.; Sikora, O.; Vitova, T.; Göttlicher, J.; Steininger, R.; Jochym, P. T.; Ptok, A.; Leupold, O.; Wille, H.-C.; Chumakov, A. I.; Piekarz, P.; Parlinski, K.; Baumbach, T.; Stankov, S.
2020. Physical review / B, 102 (19), Art.-Nr.: 195414. doi:10.1103/PhysRevB.102.195414
Kauric, G.; Walter, O.; Beck, A.; Schacherl, B.; Dieste Blanco, O.; Vigier, J.-F.; Zuleger, E.; Vitova, T.; Popa, K.
2020. Materials today advances, 8, Art.-Nr.: 100105. doi:10.1016/j.mtadv.2020.100105
Prieur, D.; Bonani, W.; Popa, K.; Walter, O.; Kriegsman, K. W.; Engelhard, M. H.; Guo, X.; Eloirdi, R.; Gouder, T.; Beck, A.; Vitova, T.; Scheinost, A. C.; Kvashnina, K.; Martin, P.
2020. Inorganic chemistry, 59 (8), 5760–5767. doi:10.1021/acs.inorgchem.0c00506
Kalt, J.; Sternik, M.; Krause, B.; Sergueev, I.; Mikolasek, M.; Bessas, D.; Sikora, O.; Vitova, T.; Göttlicher, J.; Steininger, R.; Jochym, P. T.; Ptok, A.; Leupold, O.; Wille, H.-C.; Chumakov, A. I.; Piekarz, P.; Parlinski, K.; Baumbach, T.; Stankov, S.
2020. Physical review / B, 101 (16), Art.-Nr.: 165406. doi:10.1103/PhysRevB.101.165406
Vettese, G. F.; Morris, K.; Natrajan, L. S.; Shaw, S.; Vitova, T.; Galanzew, J.; Jones, D. L.; Lloyd, J. R.
2020. Environmental science & technology, 54 (4), 2268–2276. doi:10.1021/acs.est.9b05285
Vitova, T.; Pidchenko, I.; Schild, D.; Prüßmann, T.; Montoya, V.; Fellhauer, D.; Gaona, X.; Bohnert, E.; Rothe, J.; Baker, R. J.; Geckeis, H.
2020. Inorganic chemistry, 59 (1), 8–22. doi:10.1021/acs.inorgchem.9b02463
Epifano, E.; Prieur, D.; Martin, P. M.; Guéneau, C.; Dardenne, K.; Rothe, J.; Vitova, T.; Dieste, O.; Wiss, T.; Konings, R. J. M.; Manara, D.
2020. The journal of chemical thermodynamics, 140, Article No.105896. doi:10.1016/j.jct.2019.105896
Vitova, T.; Geckeis, H.; Bagus, P. S.
2019. Actinide research quarterly, 2019 (October), 10–14
Zegke, M.; Zhang, X.; Pidchenko, I.; Hlina, J. A.; Lord, R. M.; Purkis, J.; Nichol, G. S.; Magnani, N.; Schreckenbach, G.; Vitova, T.; Love, J. B.; Arnold, P. L.
2019. Chemical science, 10 (42), 9740–9751. doi:10.1039/C8SC05717F
Neill, T. S.; Morris, K.; Pearce, C. I.; Abrahamsen-Mills, L.; Kovarik, L.; Kellet, S.; Rigby, B.; Vitova, T.; Schacherl, B.; Shaw, S.
2019. Journal of nuclear materials, 526, Article No.151751. doi:10.1016/j.jnucmat.2019.151751
Epifano, E.; Naji, M.; Manara, D.; Scheinost, A. C.; Hennig, C.; Lechelle, J.; Konings, R. J. M.; Guéneau, C.; Prieur, D.; Vitova, T.; Dardenne, K.; Rothe, J.; Martin, P. M.
2019. Communications chemistry, 2 (1), 59. doi:10.1038/s42004-019-0161-0
Rothe, J.; Altmaier, M.; Dagan, R.; Dardenne, K.; Fellhauer, D.; Gaona, X.; Corrales, E. G.-R.; Herm, M.; Kvashnina, K. O.; Metz, V.; Pidchenko, I.; Schild, D.; Vitova, T.; Geckeis, and H.
2019. Geosciences, 9 (2), Article No.91. doi:10.3390/geosciences9020091
Vitova, T.; Pidchenko, I.; Fellhauer, D.; Pruessmann, T.; Bahl, S.; Dardenne, K.; Yokosawa, T.; Schimmelpfennig, B.; Altmaier, M.; Denecke, M.; Rothe, J.; Geckeis, H.
2018. Chemical communications, 54 (91), 12824–12827. doi:10.1039/c8cc06889e
Häußler, V.; Amayri, S.; Beck, A.; Platte, T.; Stern, T. A.; Vitova, T.; Reich, T.
2018. Applied geochemistry, 98, 426–434. doi:10.1016/j.apgeochem.2018.08.021
Vitova, T.; Pidchenko, I.; Biswas, S.; Beridze, G.; Dunne, P. W.; Schild, D.; Wang, Z.; Kowalski, P. M.; Baker, R. J.
2018. Inorganic chemistry, 57 (4), 1735–1743. doi:10.1021/acs.inorgchem.7b02326
Vitova, T.
2018. Plutonium Futures: The Science 2018; Wyndham San Diego BaysideSan Diego; United States; 9 September 2018 through 14 September 2018, 377, ANS
Zimina, A.; Dardenne, K.; Denecke, M. A.; Doronkin, D. E.; Huttel, E.; Lichtenberg, H.; Mangold, S.; Pruessmann, T.; Rothe, J.; Spangenberg, T.; Steininger, R.; Vitova, T.; Geckeis, H.; Grunwaldt, J.-D.
2017. Review of scientific instruments, 88 (11), Art. Nr.: 113113. doi:10.1063/1.4999928
Bahl, S.; Peuget, S.; Pidchenko, I.; Pruessmann, T.; Rothe, J.; Dardenne, K.; Delrieu, J.; Fellhauer, D.; Jégou, C.; Geckeis, H.; Vitova, T.
2017. Inorganic chemistry, 56 (22), 13982–13990. doi:10.1021/acs.inorgchem.7b02118
Fieser, M. E.; Ferrier, M. G.; Su, J.; Batista, E.; Cary, S. K.; Engle, J. W.; Evans, W. J.; Lezama Pacheco, J. S.; Kozimor, S. A.; Olson, A. C.; Ryan, A. J.; Stein, B. W.; Wagner, G. L.; Woen, D. H.; Vitova, T.; Yang, P.
2017. Chemical science, 8 (9), 6076–6091. doi:10.1039/c7sc00825b
Vitova, T.; Pidchenko, I.; Fellhauer, D.; Bagus, P. S.; Joly, Y.; Pruessmann, T.; Bahl, S.; Gonzalez-Robles, E.; Rothe, J.; Altmaier, M.; Denecke, M. A.; Geckeis, H.
2017. Nature Communications, 8, 16053. doi:10.1038/ncomms16053
Huber, F. M.; Totskiy, Y.; Marsac, R.; Schild, D.; Pidchenko, I.; Vitova, T.; Kalmykov, S.; Geckeis, H.; Schäfer, T.
2017. Applied geochemistry, 80, 90–101. doi:10.1016/j.apgeochem.2017.01.026
Pidchenko, I.; Kvashnina, K. O.; Yokosawa, T.; Finck, N.; Bahl, S.; Schild, D.; Polly, R.; Bohnert, E.; Rossberg, A.; Göttlicher, J.; Dardenne, K.; Rothe, J.; Schäfer, T.; Geckeis, H.; Vitova, T.
2017. Environmental science & technology, 51 (4), 2217–2225. doi:10.1021/acs.est.6b04035
Polly, R.; Trumm, M.; Schimmelpfennig, B.; Tasi, A.; Gaona, X.; Pidchenko, I.; Vitova, T.; Adam, C.; Maiwald, M.; Panak, P. J.; Skerencak-Frech, A.; Geist, A.
2017. Annual Report 2016 - Institute for Nuclear Waste Disposal. Ed.: H. Geckeis, 71–74, KIT Scientific Publishing. doi:10.5445/IR/1000079683
Bahl, S.; Bauer, A.; Bohnert, E.; Dardenne, K.; González-Robles, E.; Herm, M.; Krepper, V.; Metz, V.; Pidchenko, I.; Rothe, J.; Vespa, M.; Vitova, T.
2017. Annual Report 2016 - Institute for Nuclear Waste Disposal. Ed.: H. Geckeis, 53–58, KIT Scientific Publishing. doi:10.5445/IR/1000078330
Wallesch, M.; Verma, A.; Fléchon, C.; Flügge, H.; Zink, D. M.; Seifermann, S. M.; Navarro, J. M.; Vitova, T.; Göttlicher, J.; Steininger, R.; Weinhardt, L.; Zimmer, M.; Gerhards, M.; Heske, C.; Bräse, S.; Baumann, T.; Volz, D.
2016. Chemistry - a European journal, 22 (46), 16400–16405. doi:10.1002/chem.201603847
Zimina, A.; Dardenne, K.; Denecke, M. A.; Grunwaldt, J. D.; Huttel, E.; Lichtenberg, H.; Mangold, S.; Pruessmann, T.; Rothe, J.; Steininger, R.; Vitova, T.
2016. Journal of physics / Conference Series, 712 (1), Art. Nr. 012019. doi:10.1088/1742-6596/712/1/012019
Podkovyrina, Y.; Pidchenko, I.; Prüßmann, T.; Bahl, S.; Göttlicher, J.; Soldatov, A.; Vitova, T.
2016. Journal of physics / Conference Series, 712 (1), 012092. doi:10.1088/1742-6596/712/1/012092
Pidchenko, I.; Heberling, F.; Kvashnina, K. O.; Finck, N.; Schild, D.; Bohnert, E.; Schäfer, T.; Rothe, J.; Geckeis, H.; Vitova, T.
2016. Journal of physics / Conference Series, 712, 012086/1–4. doi:10.1088/1742-6596/712/1/012086
Popa, K.; Prieur, D.; Manara, D.; Naji, M.; Vigier, J.-F.; Martin, P. M.; Blanco, O. D.; Scheinost, A. C.; Prüβmann T.; Vitova, T.; Raison, P. E.; Somers, J.; Konings, R. J. M.
2016. Dalton transactions, 45 (18), 7847–7855. doi:10.1039/C6DT00735J
Vitova, T.; Green, J. C.; Denning, R. G.; Löble, M.; Kvashnina, K.; Kas, J. J.; Jorissen, K.; Rehr, J. J.; Malcherek, T.; Denecke, M. A.
2015. Inorganic chemistry, 54, 174–182. doi:10.1021/ic5020016
Ibrahimkutty, S.; Seiler, A.; Prüßmann, T.; Vitova, T.; Pradip, R.; Bauder, O.; Wochner, P.; Plech, A.; Baumbach, T.; Stankov, S.
2015. Journal of synchrotron radiation, 22 (1), 91–98. doi:10.1107/S1600577514019705
Altmaier, M.; Bahl, S.; Bohnert, E.; Dardenne, K.; Fellhauer, D.; Gensch, A.; González-Robles, E.; Kienzler, B.; Krepper, V.; Metz, V.; Pidchenko, I.; Prüßmann, T.; Rothe, J.; Vespa, M.; Vitova, T.
2015. Annual Report 2014 / Institute for Nuclear Waste Disposal. Hrsg.: H. Geckeis, 61–65, KIT Scientific Publishing
Seiler, A.; Bauder, O.; Ibrahimkutty, S.; Pradip, R.; Prüßmann, T.; Vitova, T.; Fiederle, M.; Baumbach, T.; Stankov, S.
2014. Journal of crystal growth, 407, 74–77. doi:10.1016/j.jcrysgro.2014.09.005
Vitova, T.; Mangold, S.; Paulmann, C.; Gospodinov, M.; Marinova, V.; Mihailova, B.
2014. Physical review / B, 89, 144112/1–14. doi:10.1103/PhysRevB.89.144112
Böhler, R.; Welland, M. J.; Prieur, D.; Cakir, P.; Vitova, T.; Pruessmann, T.; Pidchenko, I.; Hennig, C.; Gueneau, C.; Konings, R. J. M.; Manara, D.
2014. Journal of nuclear materials, 448, 330–339. doi:10.1016/j.jnucmat.2014.02.029
Walshe, A.; Prüßmann, T.; Vitova, T.; Baker, R. J.
2014. Dalton transactions, 43, 4400–4407. doi:10.1039/C3DT52437J
Carvajal Nunez, U.; Eloirdi, R.; Prieur, D.; Martel, L.; Lopez Honorato, E.; Farnan, I.; Vitova, T.; Somers, J.
2014. Journal of alloys and compounds, 589, 234–239. doi:10.1016/j.jallcom.2013.11.202
Volz, D.; Wallesch, M.; Grage, S. L.; Göttlicher, J.; Steininger, R.; Batchelor, D.; Vitova, T.; Ulrich, A. S.; Heske, C.; Weinhardt, L.; Baumann, T.; Bräse, S.
2014. Inorganic chemistry frontiers, 53, 7837–7847. doi:10.1021/ic500135m
Hudry, D.; Apostolidis, C.; Walter, O.; Janen, A.; Manara, D.; Griveau, J. C.; Colineau, E.; Vitova, T.; Prüßmann, T.; Wang, D.; Kübel, C.; Meyer, D.
2014. Chemistry - a European journal, 20, 10431–10438. doi:10.1002/chem.201402008
Prüßmann, T.; Pidchenko, I.; Banik, N. L.; Dardenne, K.; Rothe, J.; Vitova, T.
2014. ANKA User Reports 2012/2013, 143–144, Karlsruher Institut für Technologie (KIT)
Bahl, S.; Kutzer, A.; Roth, G.; Geckeis; Vitova, T.
2014. ANKA User Reports 2012/2013, 137–138, Karlsruher Institut für Technologie (KIT)
Pidchenko, I.; Fellhauer, D.; Prüßmann, T.; Dardenne, K.; Rothe, J.; Vitova, T.
2014. ANKA User Reports 2012/2013, 132–133, Karlsruher Institut für Technologie (KIT)
Bube, C.; Dardenne, K.; Denecke, M. A.; Kienzler, B.; Metz, V.; Prüßmann, T.; Rothe, J.; Schild, D.; Soballa, E.; Vitova, T.
2014. ANKA User Reports 2012/2013, 30–31, Karlsruher Institut für Technologie (KIT)
Olson, A. C.; Kozimor, S. A.; Vitova, T.; Loeble, M. W.
2014. ANKA User Reports 2012/2013, 18–19, Karlsruher Institut für Technologie (KIT)
Denecke, M. A.; Petersmann, T.; Marsac, R.; Dardenne, K.; Vitova, T.; Prüßmann, T.; Borchert, M.; Bösenberg, U.; Falkenberg, G.; Wellenreuther, G.
2013. Journal of physics / Conference Series, 430, 012113/1–4. doi:10.1088/1742-6596/430/1/012113
Prüßmann, T.; Denecke, M. A.; Geist, A.; Rothe, J.; Lindqvist-Reis, P.; Löble, M.; Breher, F.; Batchelor, D. R.; Apostolidis, C.; Walter, O.; Caliebe, W.; Kvashnina, K.; Jorissen, K.; Kas, J. J.; Rehr, J. J.; Vitova, T.
2013. Journal of physics / Conference Series, 430, 012115/1–5. doi:10.1088/1742-6596/430/1/012115
Prieur, D.; Carvajal-Nunez, U.; Vitova, T.; Somers, J.
2013. European Journal of Inorganic Chemistry, (9), 1518–1524. doi:10.1002/ejic.201201294
Vitova, T.; Denecke, M. A.; Göttlicher, J.; Jorissen, K.; Kas, J. J.; Kvashnina, K.; Prüßmann, T.; Rehr, J. J.; Rothe, J.
2013. Journal of physics / Conference Series, 430, 012117/1–4. doi:10.1088/1742-6596/430/1/012117
Carvajal Nunez, U.; Martel, L.; Prieur, D.; Lopez Honorato, E.; Eloirdi, R.; farnan, I.; Vitova, T.; Somers, J.
2013. Inorganic Chemistry, 52, 11669–11676. doi:10.1021/ic402144g
Löble, M. W.; Ona-Burgos, P.; Fernández, I.; Apostolidis, C.; Morgenstern, A.; Walter, O.; Bruchertseifer, F.; Kaden, P.; Vitova, T.; Rothe, J.; Dardenne, K.; Banik, N. L.; Geist, A.; Denecke, M. A.; Breher, F.
2013. Chemical science, 4 (9), 3717–3724. doi:10.1039/C3SC50708D
Göttlicher, J.; Kotelnikov, A.; Suk, N.; Kovalski, A.; Vitova, T.; Steininger, R.
2013. Zeitschrift für Kristallographie, 228, 157–171. doi:10.1524/zkri.2013.1587
Rothe, J.; Brendebach, B.; Bube, C.; Dardenne, K.; Denecke, M. A.; Kienzler, B.; Metz, V.; Prüßmann, T.; Rickers-Appel, K.; Schild, D.; Soballe, E.; Vitova, T.
2013. Journal of Physics: Conference Series, 430, 012114/1–5. doi:10.1088/1742-6596/430/1/012114
Batuk, O. N.; Szabo, D. V.; Denecke, M. A.; Vitova, T.; Kalmykov, S. N.
2013. Radiochimica acta, 101 (4), 233–239. doi:10.1524/ract.2012.2014
Bube, C.; Dardenne, K.; Denecke, M. A.; Fröhlich, D. R.; Kienzler, B.; Metz, V.; Panak, P. J.; Prüßmann, T.; Rothe, J.; Schild, D.; Skerencak, A.; Soballa, E.; Vitova, T.
2013. Annual Report 2012 : Institute for Nuclear Waste Disposal. Ed.: H. Geckeis, 77–83, KIT Scientific Publishing
Kutzer, A.; Vitova, T.; Kvashnina, K.; Prüßmann, T.; Rothe, J.; Adam, C.; Kaden, P.; Denecke, M. A.; Weisenburger, S.; Roth, G.; Geckeis, H.
2013. Annual Report 2012 : Institute for Nuclear Waste Disposal. Ed.: H. Geckeis, 73–75, KIT Scientific Publishing
Carvajal-Nunez, U.; Prieur, D.; Vitova, T.; Somers, J.
2012. Inorganic Chemistry, 51 (21), 11762–11768. doi:10.1021/ic301709d
Huber, F.; Schild, D.; Vitova, T.; Rothe, J.; Kirsch, R.; Schäfer, T.
2012. Geochimica et Cosmochimica Acta, 96, 154–173. doi:10.1016/j.gca.2012.07.019
Vespa, M.; Rini, M.; Spino, J.; Vitova, T.; Somers, J.
2012. Journal of Nuclear Materials, 421, 80–88. doi:10.1016/j.jnucmat.2011.11.055
Rothe, J.; Butorin, S.; Dardenne, K.; Denecke, M. A.; Kienzler, B.; Löble, M.; Metz, V.; Seibert, A.; Steppert, M.; Vitova, T.; Walther, C.; Geckeis, H.
2012. Review of Scientific Instruments, 83, 043105/1–13. doi:10.1063/1.3700813
Denecke, M. A.; Borchert, M.; Denning, R. G.; De Nolf, W.; Falkenberg, G.; Hon̈ig S.; Klinkenberg, M.; Kvashnina, K.; Neumeier, S.; Patommel, J.; Petersmann, T.; Pruessmann, T.; Ritter, S.; Schroer, C. G.; Stephan, S.; Villanova, J.; Vitova, T.; Wellenreuther, G.
2012. MRS online proceedings library, 1444 (1), 269–280. doi:10.1557/opl.2012.1159
Vitova, T.; Denecke, M. A.; Finck, N.; Göttlicher, J.; Kienzler, B.; Rothe, J.
2012. 2nd Internat.Workshop on Actinide Brine Chemistry in a Salt-Based Repository (ABC-SALT (II)), Karlsruhe, November 7-8, 2011, 107–108, KIT Scientific Publishing
Huber, F. M.; Schild, D.; Vitova, T.; Rothe, J.; Kirsch, R.; Schäfer, T.
2012. 4th Annual Workshop Proceedings of the Collaborative Project "Redox Phenomena Controlling Systems" (7th EC FP CP RECOSY). Ed.: M. Altmaier, 383–397, KIT Scientific Publishing
Pidchenko, I.; Salminen-Paatero, S.; Vitova, T.; Suksi, J.
2012. 4th Annual Workshop Proceedings of the Collaborative Project "Redox Phenomena Controlling Systems" (7th EC FP CP RECOSY). Ed.: M. Altmaier, 223–230, KIT Scientific Publishing
Vitova, T.; Butorin, S. M.; Seibert, A.; Rothe, J.; Dardenne, K.; Vegelius, J.; Caciuffo, R.; Denecke, M. A.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 394–395
Löble, M.; Vitova, T.; Brendebach, B.; Rothe, J.; Dardenne, K.; Denecke, M. A.; Breher, F.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 337–338
Li, B.; Dardenne, K.; Vitova, T.; Rothe, J.; Foerstendorf, H.; Raff, J.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 379
Kutzer, A.; Vitova, T.; Denecke, M. A.; Roth, G.; Geckeis, H.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 336
Vitova, T.; Huber, F.; Rothe, J.; Dardenne, K.; Schäfer, T.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 329–330
Schepperle, J.; Finck, N.; Vitova, T.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 327–328
Vitova, T.; Dardenne, K.; Denecke, M. A.; Ernst, H.; Rothe, J.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 326
Butorin, S. M.; Vitova, T.; Vegelius, J.; Seibert, A.; Caciuffo, R.; Denecke, M. A.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 295–296
Löble, M.; Vitova, T.; Brendebach, B.; Rothe, J.; Dardenne, K.; Denecke, M. A.; Breher, F.
2012. ANKA - Annual Report 2010/2011 Karlsruhe : Karlsruhe Institute of Technology, 2012 Also publ.online, 307–309
Collaborations
Lawrence Berkeley National Laboratory, USA |
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Polly Arnold https://chemistry.berkeley.edu/faculty/chem/polly-arnold Stefan Minasian https://profiles.lbl.gov/20637-stefan-minasian
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Deutsches Krebsforschungszentrum Heidelberg, Germany |
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Martina Benešová-Schäfer |
Pacific Northwest National Laboratory (PNNL), USA |
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Jennifer Yao Eugene Ilton Bruce K. McNamara Edgar C. Buck |
Los Alamos National Laboratory, USA |
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Stosh Kozimor Ping Yang Enrique Batista |
École Polytechnique Fédérale de Lausanne, Switzerland |
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Marinella Mazzanti Rizlan Bernier-Latmani |
University of Manchester, UK |
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Katherine Morris Samuel Shaw Tom Neill |
European Synchrotron Radiation Facility, France |
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Kristina Kvashnina https://www.esrf.eu/home/Members/content/staff-web-pages/kvashnin.html |
CEA, DEN, DEC, CEN Cadarache, France |
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Philippe Martin |
Joint Research Center-Karlsruhe, Germany |
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Thiery Wiss Olaf Walter Karin Popa Antonio Bulgheroni Rachel Eloirdi Attila Kovács Alice Seibert |
Uppsala University, Sweden |
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Sergei M. Butorin |
Heidelberg University, Germany |
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Maurits Haverkort |
Contact us!
If you are looking for a bachelor, master or PhD project with exciting topic including application of novel synchrotron based X-ray spectroscopy methods contact us. You will have the opportunity to reveal structural properties of actinide and lanthanide systems important for example for molecular scale understanding of processes in a nuclear waste repository. You will work in a young, motivated and enthusiastic team and will perform experiments at the KIT Light Source and other national and international synchrotron radiation facilities.
| Email: | Tonya.Vitova∂kit.edu |
| Telephone: | +49 721 608 24024 |
| Address: | Karlsruhe Institute of Technology Institute for Nuclear Waste Disposal Hermann von Helmholtz Platz 1 76344 Eggenstein-Leopoldshafen, Germany |